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Sensitivity analysis of the deterioration of concrete strength in marine environment to multiple corrosive ions

《结构与土木工程前沿（英文）》 2023年 第17卷 第2期   页码 175-190 doi: 10.1007/s11709-021-0791-z

摘要： The corrosion degradation behavior of concrete materials plays a crucial role in the change of its mechanical properties under multi-ion interaction in the marine environment. In this study, the variation in the macro-physical and mechanical properties of concrete with corrosion time is investigated, and the source of micro-corrosion products under different salt solutions in seawater are analyzed. Regardless of the continuous hydration effect of concrete, the damage effects of various corrosive ions (Cl–, SO42−, and Mg2+, etc.) on the tensile and compressive strength of concrete are discussed based on measurement in different salt solutions. The sensitivity analysis method for concrete strength is used to quantitatively analyze the sensitivity of concrete strength to the effects of each ion in a multi-salt solution without considering the influence of continued hydration. The quantitative results indicate that the addition of Cl– can weaken the corrosion effect of SO42− by about 20%, while the addition of Mg2+ or Mg2+ and Cl– can strengthen it by 10%–20% during a 600-d corrosion process.

关键词： sensitivity analysis     concrete strength     corrosion deterioration     multi-ion interaction     marine environment    

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Multi-effect anthraquinone-based polyimide enclosed SnO/reduced graphene oxide composite as high-performanceanode for lithium-ion battery

《化学科学与工程前沿（英文）》 2023年 第17卷 第9期   页码 1231-1243 doi: 10.1007/s11705-023-2306-z

摘要： The cycling stability of SnO2 anode as lithium-ion battery is poor due to volume expansion. Polyimide coatings can effectively confine the expansion of SnO2. However, linear polyimides are easily dissolved in ester electrolytes and their carbonyls is not fully utilized during charging/discharging process. Herein, the SnO2 enclosed with anthraquinone-based polyimide/reduced graphene oxide composite was prepared by self-assembly. Carbonyls from the anthraquinone unit provide fully available active sites to react with Li+, improving the utilization of carbonyl in the polyimide. More exposed carbonyl active sites promote the conversion of Sn to SnO2 with electrode gradual activation, leading to an increase in reversible capacity during the charge/discharge cycle. In addition, the introduction of reduced graphene oxide cannot only improve the stability of polyimide in the electrolyte, but also build fast ion and electron transport channels for composite electrodes. Due to the multiple effects of anthraquinone-based polyimide and the synergistic effect of reducing graphene oxide, the composite anode exhibits a maximum reversible capacity of 1266 mAh·g−1 at 0.25 A·g−1, and maintains an excellent specific capacity of 983 mAh·g−1 after 200 cycles. This work provides a new strategy for the synergistic modification of SnO2.

关键词： anthraquinone-based polyimide     multi-effect     tin dioxide     reduced graphene oxide     lithium-ion battery    

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A method of determining flame radiation fraction induced by interaction burning of tri-symmetric propanefires in open space based on weighted multi-point source model

Jie JI, Junrui DUAN, Huaxian WAN

《能源前沿（英文）》 2022年 第16卷 第6期   页码 1017-1026 doi: 10.1007/s11708-020-0716-x

摘要： The interaction of multiple fires may lead to a higher flame height and more intense radiation flux than a single fire, which increases the possibility of flame spread and risks to the surroundings. Experiments were conducted using three burners with identical heat release rates (HRRs) and propane as the fuel at various spacings. The results show that flames change from non-merging to merging as the spacing decreases, which result in a complex evolution of flame height and merging point height. To facilitate the analysis, a novel merging criterion based on the dimensionless spacing / was proposed. For non-merging flames ( / >0.368), the flame height is almost identical to a single fire; for merging flames ( / ≤0.368), based on the relationship between thermal buoyancy and thrust (the pressure difference between the inside and outside of the flame), a quantitative analysis of the flame height, merging point height, and air entrainment was formed, and the calculated merging flame heights show a good agreement with the measured experimental values. Moreover, the multi-point source model was further improved, and radiation fraction of propane was calculated. The data obtained in this study would play an important role in calculating the external radiation of propane fire.

关键词： flame interaction     air entrainment     flame height     multi-point source model     thermal radiation    

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Removable Dyes—The Missing Link for In-Depth N-glycan Analysis via Multi-Method Approaches

Samanta Cajic,René Hennig,Valerian Grote,Udo Reichl,Erdmann Rapp,

《工程（英文）》 doi: 10.1016/j.eng.2023.02.016

摘要： As the roles of glycans in health and disease continue to be unraveled, it is becoming apparent that glycans’ immense complexity cannot be ignored. To fully delineate glycan structures, we developed an integrative approach combining a set of cost-effective, widespread, and easy-to-handle analytical methods. The key feature of our workflow is the exploitation of a removable fluorescent label—exemplified by 9-fluorenylmethyl chloroformate (Fmoc)—to bridge the gap between diverse glycoanalytical methods, especially multiplexed capillary gel electrophoresis with laser-induced fluorescence detection (xCGE-LIF) and matrix-assisted laser desorption/ionization time-of-flight mass spectrometry (MALDI-TOF-MS). Through the detailed structural analysis of selected, dauntingly complex N-glycans from chicken ovalbumin, horse serum, and bovine transferrin, we illustrate the capabilities of the presented strategy. Moreover, this approach “visualizes” N-glycans that have been difficult to identify thus far—such as the sulfated glycans on human immunoglobulin A—including minute changes in glycan structures, potentially providing useful new targets for biomarker discovery.

关键词： Glycoproteins     N-glycans     Reversible labeling     Hydrophilic interaction liquid chromatography     Capillary gel electrophoresis     Mass spectrometry    

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Advancing ion-exchange membranes to ion-selective membranes: principles, status, and opportunities

《环境科学与工程前沿（英文）》 2023年 第17卷 第2期 doi: 10.1007/s11783-023-1625-0

摘要：

● IEM ion/ion selectivities of charge, valence, & specific ion are critically assessed.

关键词： Ion-exchange membranes     Selectivity     Separations    

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Interaction of carbonaceous nanomaterials with wastewater biomass

Yu YANG,Zhicheng YU,Takayuki NOSAKA,Kyle DOUDRICK,Kiril HRISTOVSKI,Pierre HERCKES,Paul WESTERHOFF

《环境科学与工程前沿（英文）》 2015年 第9卷 第5期   页码 823-831 doi: 10.1007/s11783-015-0787-9

摘要： Increasing production and use of carbonaceous nanomaterials (NMs) will increase their release to the sewer system and to municipal wastewater treatment plants. There is little quantitative knowledge on the removal of multi-walled carbon nanotubes (MWCNTs), graphene oxide (GO), or few-layer graphene (FLG) from wastewater into the wastewater biomass. As such, we investigated the quantification of GO and MWCNTs by UV-Vis spectrophotometry, and FLG using programmable thermal analysis (PTA), respectively. We further explored the removal of pristine and oxidized MWCNTs (O-MWCNTs), GO, and FLG in a biomass suspension. At least 96% of pristine and O-MWCNTs were removed from the water phase through aggregation and 30-min settling in presence or absence of biomass with an initial MWCNT concentration of 25 mg·L . Only 65% of GO was removed with biomass concentration at or above 1,000 mg·L as total suspended solids (TSS) with the initial GO concentration of 25 mg·L . As UV-Vis spectrophotometry does not work well on quantification of FLG, we studied the removal of FLG at a lower biomass concentration (50 mg TSS·L ) using PTA, which showed a 16% removal of FLG with an initial concentration of 1 mg·L . The removal data for GO and FLG were fitted using the Freundlich equation ( = 0.55, 0.94, respectively). The data presented in this study for carbonaceous NM removal from wastewater provides quantitative information for environmental exposure modeling and life cycle assessment.

关键词： multi-walled carbon nanotubes     graphene oxide     graphene     removal     wastewater biomass    

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Advances in crop phenotyping and multi-environment trials

Zhe LIU,Fan ZHANG,Qin MA,Dong AN,Lin LI,Xiaodong ZHANG,Dehai ZHU,Shaoming LI

《农业科学与工程前沿（英文）》 2015年 第2卷 第1期   页码 28-37 doi: 10.15302/J-FASE-2015051

摘要： Efficient evaluation of crop phenotypes is a prerequisite for breeding, cultivar adoption, genomics and phenomics study. Plant genotyping is developing rapidly through the use of high-throughput sequencing techniques, while plant phenotyping has lagged far behind and it has become the rate-limiting factor in genetics, large-scale breeding and development of new cultivars. In this paper, we consider crop phenotyping technology under three categories. The first is high-throughput phenotyping techniques in controlled environments such as greenhouses or specifically designed platforms. The second is a phenotypic strengthening test in semi-controlled environments, especially for traits that are difficult to be tested in multi-environment trials (MET), such as lodging, drought and disease resistance. The third is MET in uncontrolled environments, in which crop plants are managed according to farmer’s cultural practices. Research and application of these phenotyping techniques are reviewed and methods for MET improvement proposed.

关键词： crop breeding     genotyping     phenotyping     genotype-environment interaction     cultivar regional test    

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Review of pantograph and catenary interaction

Weihua ZHANG, Dong ZOU, Mengying TAN, Ning ZHOU, Ruiping LI, Guiming MEI

《机械工程前沿（英文）》 2018年 第13卷 第2期   页码 311-322 doi: 10.1007/s11465-018-0494-x

摘要：

The application of electrified railway directly promotes relevant studies on pantograph-catenary interaction. With the increase of train running speed, the operating conditions for pantograph and catenary have become increasingly complex. This paper reviews the related achievements contributed by groups and institutions around the world. This article specifically focuses on three aspects: The dynamic characteristics of the pantograph and catenary components, the systems’ dynamic properties, and the environmental influences on the pantograph-catenary interaction. In accordance with the existing studies, future research may prioritize the task of identifying the mechanism of contact force variation. This kind of study can be carried out by simplifying the pantograph-catenary interaction into a moving load problem and utilizing the theory of matching mechanical impedance. In addition, developing a computational platform that accommodates environmental interferences and multi-field coupling effects is necessary in order to further explore applications based on fundamental studies.

关键词： electrified railway     pantograph and catenary interaction     contact force variation     moving load problem     mechanical impedance     multi-field    

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Alumina modified sodium vanadate cathode for aqueous zinc-ion batteries

《能源前沿（英文）》   页码 775-781 doi: 10.1007/s11708-023-0902-8

摘要： Aqueous zinc-ion batteries (ZIBs) have great prospects for widespread application in massive scale energy storage. By virtue of the multivalent state, open frame structure and high theoretical specific capacity, vanadium (V)-based compounds are a kind of the most developmental potential cathode materials for ZIBs. However, the slow kinetics caused by low conductivity and the capacity degradation caused by material dissolution still need to be addressed for large-scale applications. Therefore, sodium vanadate Na2V6O16·3H2O (NVO) was chosen as a model material, and was modified with alumina coating through simple mixing and stirring methods. After Al2O3 coating modification, the rate capability and long-cycle stability of Zn//NVO@Al2O3 battery have been significantly improved. The discharge specific capacity of NVO@Al2O3 reach up to 228 mAh/g (at 4 A/g), with a capacity reservation rate of approximately 68% after 1000 cycles, and the Coulombic efficiency (CE) is close to 100%. As a comparison, the capacity reservation rate of Zn//NVO battery is only 27.7%. Its superior electrochemical performance is mainly attributed to the Al2O3 coating layer, which can increase zinc-ion conductivity of the material surface, and to some extent inhibit the dissolution of NVO, making the structure stable and improving the cyclic stability of the material. This paper offers new prospects for the development of cathode coating materials for ZIBs.

关键词： cathodes     aqueous zinc-ion batteries     sodium vanadate     alumina     coating    

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Reactive power compensation of an isolated hybrid power system with load interaction using ANFIS tuned

Nitin SAXENA,Ashwani KUMAR

《能源前沿（英文）》 2014年 第8卷 第2期   页码 261-268 doi: 10.1007/s11708-014-0298-6

摘要： This paper presents an adaptive neuro fuzzy interference system (ANFIS) based approach to tune the parameters of the static synchronous compensator (STATCOM) with frequent disturbances in load model and power input of a wind-diesel based isolated hybrid power system (IHPS). In literature, proportional integral (PI) based controller constants are optimized for voltage stability in hybrid systems due to the interaction of load disturbances and input power disturbances. These conventional controlling techniques use the integral square error (ISE) criterion with an open loop load model. An ANFIS tuned constants of a STATCOM controller for controlling the reactive power requirement to stabilize the voltage variation is proposed in the paper. Moreover, the interaction between the load and the isolated power system is developed in terms of closed loop load interaction with the system. Furthermore, a comparison of transient responses of IHPS is also presented when the system has only the STATCOM and the static compensation requirement of the induction generator is fulfilled by the fixed capacitor, dynamic compensation requirement, meanwhile, is fulfilled by STATCOM. The model is tested for a 1% step increase in reactive power load demand at = 0 s and then a sudden change of 3% from the 1% at = 0.01 s for a 1% step increase in power input at variable wind speed model.

关键词： isolated wind-diesel power system     adaptive neuro fuzzy interference system (ANFIS)     integral square error (ISE) criterion     load interaction    

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Vanadium oxide cathode with synergistic engineering of calcium-ion intercalation and polyaniline coatingfor high performance zinc-ion batteries

《化学科学与工程前沿（英文）》 2023年 第17卷 第9期   页码 1244-1253 doi: 10.1007/s11705-022-2293-5

摘要： Vanadium oxides as cathode for zinc-ion batteries have attracted much attention because of their high theoretical capacity, flexible layered structure and abundant resources. However, cathodes are susceptible to the collapse of their layered structure and the dissolution of vanadium after repeated long cycles, which worsen their capacities and cycling stabilities. Herein, a synergistic engineering of calcium-ion intercalation and polyaniline coating was developed to achieve the superior electrochemical performance of vanadium pentoxide for zinc-ion batteries. The pre-intercalation of calcium-ion between vanadium pentoxide layers as pillars increase the crystal structure’s stability, while the polyaniline coating on the cathodes improves the conductivity and inhibits the dissolution of vanadium. This synergistic engineering enables that the battery system based-on the polyaniline coated calcium vanadate cathode to deliver a high capacity of 406.4 mAh·g−1 at 1 A·g−1, an ultralong cycle life over 6000 cycles at 10 A·g−1 with 93% capacity retention and high-rate capability. The vanadium oxide cathode with synergistic engineering of calcium-ion intercalation and polyaniline coating was verified to effectively improve the electrochemical performance of zinc-ion batteries.

关键词： zinc-ion battery     CaV8O20     polyaniline coating     synergistic engineering     high capacity     long durability    

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An efficient method for the dynamic interaction of open structure-foundation systems

LIU Jingbo, GU Yin, LI Bin, WANG Yan

《结构与土木工程前沿（英文）》 2007年 第1卷 第3期   页码 340-345 doi: 10.1007/s11709-007-0045-8

摘要： The structure-foundation system is transformed from an original open system into an approximately hermetic system through a viscous-spring artificial boundary. In addition, the seismic wave scattering problem is changed to a wave source problem by employing an equivalent seismic wave input method. Subsequently, the modal superposition method is adopted to solve the approximated hermetic system. This procedure is highly efficient in analyzing dynamic structure-foundation interaction problems in the time domain. Two numerical examples are presented to illustrate the characteristics of the proposed method: one is a wave source problem in 2-dimensions (2-D) elastic semi-infinite space, and the other is a dynamic structure-foundation interaction problem under seismic excitations. Compared with the traditional direct step-by-step integration method, the proposed method, with a sufficient number of modes included, can significantly reduce the computational time with almost the same precision. The results also indicate that the proposed method is more advantageous for solving large structure-foundation systems of many degrees of freedom.

关键词： structure-foundation interaction     superposition     interaction problem     freedom     efficient    

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Ion-imprinted silica gel and its dynamic membrane for nickel ion removal from wastewaters

Jiehui Zeng, Jianxian Zeng, Hu Zhou, Guoqing Liu, Zhengqiu Yuan, Jian Jian

《化学科学与工程前沿（英文）》 2020年 第14卷 第6期   页码 1018-1028 doi: 10.1007/s11705-020-1915-z

摘要： An ion-imprinted sorbent (IIP) was prepared by using Ni as template, 3-[2-(2-aminoethylamino) ethylamino] propyl-trimethoxysilane as functional monomer, and silica gel as carrier. The adsorption performance of IIP towards Ni was investigated. IIP showed a higher adsorption capacity than that of non-imprinted sorbent, and it also exhibited high selectivity for Ni in the presence of Cu and Zn ions. Then, IIP was used to form a dynamic membrane onto the surface of ceramic membrane for treatment of electroplating wastewater containing Ni . Compared with ceramic membrane, IIP dynamic membrane had much higher steady membrane flux, and also rejected Ni to obtain a lower concentration of Ni in the permeate fluid. Perhaps it is suitable for future practice applications.

关键词： ion-imprinted     nickel ion     dynamic membrane     adsorption    

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Systems understanding of plant–pathogen interactions through genome-wide protein–protein interaction

Hong LI,Ziding ZHANG

《农业科学与工程前沿（英文）》 2016年 第3卷 第2期   页码 102-112 doi: 10.15302/J-FASE-2016100

摘要： Plants are frequently affected by pathogen infections. To effectively defend against such infections, two major modes of innate immunity have evolved in plants; pathogen-associated molecular pattern-triggered immunity and effector-triggered immunity. Although the molecular components as well as the corresponding pathways involved in these two processes have been identified, many aspects of the molecular mechanisms of the plant immune system remain elusive. Recently, the rapid development of omics techniques (e.g., genomics, proteomics and transcriptomics) has provided a great opportunity to explore plant–pathogen interactions from a systems perspective and studies on protein–protein interactions (PPIs) between plants and pathogens have been carried out and characterized at the network level. In this review, we introduce experimental and computational identification methods of PPIs, popular PPI network analysis approaches, and existing bioinformatics resources/tools related to PPIs. Then, we focus on reviewing the progress in genome-wide PPI networks related to plant–pathogen interactions, including pathogen-centric PPI networks, plant-centric PPI networks and interspecies PPI networks between plants and pathogens. We anticipate genome-wide PPI network analysis will provide a clearer understanding of plant–pathogen interactions and will offer some new opportunities for crop protection and improvement.

关键词： plant–pathogen interactions     systems biology     omics     plant immunity     protein–protein interaction     network    

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Highly selective metal recovery from spent lithium-ion batteries through stoichiometric hydrogen ion

Weiguang Lv, Xiaohong Zheng, Li Li, Hongbin Cao, Yi Zhang, Renjie Chen, Hancheng Ou, Fei Kang, Zhi Sun

《化学科学与工程前沿（英文）》 2021年 第15卷 第5期   页码 1243-1256 doi: 10.1007/s11705-020-2029-3

摘要： Spent lithium-ion battery recycling has attracted significant attention because of its importance in regard to the environment and resource importance. Traditional hydrometallurgical methods usually leach all valuable metals and subsequently extract target meals to prepare corresponding materials. However, Li recovery in these processes requires lengthy operational procedures, and the recovery efficiency is low. In this research, we demonstrate a method to selectively recover lithium before the leaching of other elements by introducing a hydrothermal treatment. Approximately 90% of Li is leached from high-Ni layered oxide cathode powders, while consuming a nearly stoichiometric amount of hydrogen ions. With this selective recovery of Li, the transition metals remain as solid residue hydroxides or oxides. Furthermore, the extraction of Li is found to be highly dependent on the content of transition metals in the cathode materials. A high leaching selectivity of Li (>98%) and nearly 95% leaching efficiency of Li can be reached with LiNi Co Mn O . In this case, both the energy and material consumption during the proposed Li recovery is significantly decreased compared to traditional methods; furthermore, the proposed method makes full use of H to leach Li . This research is expected to provide new understanding for selectively recovering metal from secondary resources.

关键词： recycling     spent LIBs     selective recovery     hydrothermal treatment    

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标题 作者 时间 类型 操作

Sensitivity analysis of the deterioration of concrete strength in marine environment to multiple corrosive ions

期刊论文

Multi-effect anthraquinone-based polyimide enclosed SnO/reduced graphene oxide composite as high-performanceanode for lithium-ion battery

期刊论文

A method of determining flame radiation fraction induced by interaction burning of tri-symmetric propanefires in open space based on weighted multi-point source model

Jie JI, Junrui DUAN, Huaxian WAN

期刊论文

Removable Dyes—The Missing Link for In-Depth N-glycan Analysis via Multi-Method Approaches

Samanta Cajic,René Hennig,Valerian Grote,Udo Reichl,Erdmann Rapp,

期刊论文

Advancing ion-exchange membranes to ion-selective membranes: principles, status, and opportunities

期刊论文

Interaction of carbonaceous nanomaterials with wastewater biomass

Yu YANG,Zhicheng YU,Takayuki NOSAKA,Kyle DOUDRICK,Kiril HRISTOVSKI,Pierre HERCKES,Paul WESTERHOFF

期刊论文

Advances in crop phenotyping and multi-environment trials

Zhe LIU,Fan ZHANG,Qin MA,Dong AN,Lin LI,Xiaodong ZHANG,Dehai ZHU,Shaoming LI

期刊论文

Review of pantograph and catenary interaction

Weihua ZHANG, Dong ZOU, Mengying TAN, Ning ZHOU, Ruiping LI, Guiming MEI

期刊论文

Alumina modified sodium vanadate cathode for aqueous zinc-ion batteries

期刊论文

Reactive power compensation of an isolated hybrid power system with load interaction using ANFIS tuned

Nitin SAXENA,Ashwani KUMAR

期刊论文

Vanadium oxide cathode with synergistic engineering of calcium-ion intercalation and polyaniline coatingfor high performance zinc-ion batteries

期刊论文

An efficient method for the dynamic interaction of open structure-foundation systems

LIU Jingbo, GU Yin, LI Bin, WANG Yan

期刊论文

Ion-imprinted silica gel and its dynamic membrane for nickel ion removal from wastewaters

Jiehui Zeng, Jianxian Zeng, Hu Zhou, Guoqing Liu, Zhengqiu Yuan, Jian Jian

期刊论文

Systems understanding of plant–pathogen interactions through genome-wide protein–protein interaction

Hong LI,Ziding ZHANG

期刊论文

Highly selective metal recovery from spent lithium-ion batteries through stoichiometric hydrogen ion

Weiguang Lv, Xiaohong Zheng, Li Li, Hongbin Cao, Yi Zhang, Renjie Chen, Hancheng Ou, Fei Kang, Zhi Sun

期刊论文